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    Influence of activated carbon surface oxygen functionalities on SO2 physisorption – Simulation and experiment

    192581_192561.pdf (1.309Mb)
    Access Status
    Open access
    Authors
    Furmaniak, S.
    Terzyk, A.
    Gauden, P.
    Kowalczyk, Piotr
    Szymanski, G.
    Date
    2013
    Type
    Journal Article
    
    Metadata
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    Citation
    Furmaniak, Sylwester and Terzyk, Artur P. and Gauden, Piotr A. and Kowalczyk, Piotr and Szymanski, Grzegorz S.. 2013. Influence of activated carbon surface oxygen functionalities on SO2 physisorption – Simulation and experiment. Chemical Physics Letters. 578: pp. 85-91.
    Source Title
    Chemical Physics Letters
    DOI
    10.1016/j.cplett.2013.05.060
    ISSN
    0009-2614
    URI
    http://hdl.handle.net/20.500.11937/18934
    Collection
    • Curtin Research Publications
    Abstract

    The influence of the gradual oxidation of carbons on SO2 physisorption was studied, by comparison of experimental and simulated SO2 adsorption isotherms. The results confirmed a significant impact of surface groups on the SO2 adsorption. The simulations also revealed a similar, to that observed experimentally, effect of the increase in the percentage of the smallest micropores on adsorption isotherms. The isotherms were analysed using the CMMS model. The conclusion is that this model seems to be a good and sensitive tool for studying SO2 physisorption mechanism since a very good qualitative agreement between the experimental and simulated data was observed.

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