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    The lead pollution history of Law Dome, Antarctica, from isotopic measurements on ice cores: 1500 AD to 1989 AD

    Access Status
    Fulltext not available
    Authors
    Vallelonga, Paul
    Van de Velde, Katja
    Candelone, Jean
    Morgan, V.
    Boutron, C.
    Rosman, Kevin
    Date
    2002
    Type
    Journal Article
    
    Metadata
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    Citation
    Vallelonga, Paul and Van De Velde, Katja and Candelone, Jean and Morgan, V. and Boutron, C. and Rosman, Kevin. 2002. The lead pollution history of Law Dome, Antarctica, from isotopic measurements on ice cores: 1500 AD to 1989 AD. Earth and Planetary Science Letters. 204 (1-2): pp. 291-306.
    Source Title
    Earth and Planetary Science Letters
    DOI
    10.1016/S0012-821X(02)00983-4
    ISSN
    0012821X
    Faculty
    Department of Medical Imaging and Applied Physics
    School of Science
    Faculty of Science and Engineering
    School
    Department of Imaging and Applied Physics
    Remarks

    The link to the journal’s home page is: http://www.elsevier.com/wps/find/journaldescription.cws_home/503328/description#description

    Copyright © 2002 Elsevier Ltd. All rights reserved

    URI
    http://hdl.handle.net/20.500.11937/35678
    Collection
    • Curtin Research Publications
    Abstract

    Lead isotopic compositions and Pb and Ba concentrations have been measured in ice cores from Law Dome, East Antarctica, covering the past 6500 years. ‘Natural’ background concentrations of Pb (0.4 pg/g) and Ba (1.3 pg/g) are observed until 1884 AD, after which increased Pb concentrations and lowered 206Pb/207Pb ratios indicate the influence of anthropogenic Pb. The isotopic composition of ‘natural’ Pb varies within the range 206Pb/207Pb=1.20–1.25 and 208Pb/207Pb=2.46–2.50, with an average rock and soil dust Pb contribution of 8–12%. A major pollution event is observed at Law Dome between 1884 and 1908 AD, elevating the Pb concentration four-fold and changing 206Pb/207Pb ratios in the ice to 1.12. Based on Pb isotopic systematics and Pb emission statistics, this is attributed to Pb mined at Broken Hill and smelted at Broken Hill and Port Pirie, Australia. Anthropogenic Pb inputs are at their greatest from 1900 to 1910 and from 1960 to 1980. During the 20th century, Ba concentrations are consistently higher than ‘natural’ levels and are attributed to increased dust production, suggesting the influence of climate change and/or changes in land coverage with vegetation.

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