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dc.contributor.authorLi, C.
dc.contributor.authorShi, Y.
dc.contributor.authorZhang, H.
dc.contributor.authorZhao, Q.
dc.contributor.authorXue, F.
dc.contributor.authorLi, Xin Yong
dc.date.accessioned2017-01-30T14:57:09Z
dc.date.available2017-01-30T14:57:09Z
dc.date.created2016-07-06T19:30:16Z
dc.date.issued2016
dc.identifier.citationLi, C. and Shi, Y. and Zhang, H. and Zhao, Q. and Xue, F. and Li, X.Y. 2016. Cu-BTC metal-organic framework as a novel catalyst for low temperature selective catalytic reduction (SCR) of NO by NH3: Promotional effect of activation temperature. Integrated Ferroelectrics. 172 (1): pp. 169-179.
dc.identifier.urihttp://hdl.handle.net/20.500.11937/42055
dc.identifier.doi10.1080/10584587.2016.1177385
dc.description.abstract

Metal-organic framework Cu-BTC was synthesized by hydrothermal method, and was employed as denitrification catalyst for low temperature selective catalytic reduction of NO with NH3 (NH3-SCR). After activated at different temperatures from 180°C to 250°C in vacuum, Cu-BTC samples were characterized by NH3-SCR test, X-ray powder diffraction, thermal analysis, scanning electron microscope and in situ Fourier-transform infrared. NO conversion results revealed that activation temperatures played a significant beneficial effect role in Cu-BTC catalytic performance for low-temperature NH3-SCR reaction. The Cu-BTC catalyst pre-treated at 230°C achieved a complete NO conversion efficiency with large operating-temperature window from 220°C to 280°C. This excellent catalytic activity was mainly attributed to the unsaturated Cu sites in Cu-BTC. The correlation between catalytic property and structure of Cu-BTC was discussed.

dc.titleCu-BTC metal-organic framework as a novel catalyst for low temperature selective catalytic reduction (SCR) of NO by NH3: Promotional effect of activation temperature
dc.typeJournal Article
dcterms.source.volume172
dcterms.source.number1
dcterms.source.startPage169
dcterms.source.endPage179
dcterms.source.issn1058-4587
dcterms.source.titleIntegrated Ferroelectrics
curtin.departmentDepartment of Chemical Engineering
curtin.accessStatusFulltext not available


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