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    Thermal Conversion of Core-Shell Metal-Organic Frameworks: A New Method for Selectively Functionalized Nanoporous Hybrid Carbon

    Access Status
    Fulltext not available
    Authors
    Tang, J.
    Salunkhe, R.
    Liu, Jian
    Torad, N.
    Imura, M.
    Furukawa, S.
    Yamauchi, Y.
    Date
    2015
    Type
    Journal Article
    
    Metadata
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    Citation
    Tang, J. and Salunkhe, R. and Liu, J. and Yamauchi, Y. 2015. Thermal Conversion of Core-Shell Metal-Organic Frameworks: A New Method for Selectively Functionalized Nanoporous Hybrid Carbon. Journal of the American Chemical Society. 137: pp. 1572-1580.
    Source Title
    Journal of the American Chemical Society
    DOI
    10.1021/ja511539a
    ISSN
    0002-7863
    School
    Department of Chemical Engineering
    URI
    http://hdl.handle.net/20.500.11937/5223
    Collection
    • Curtin Research Publications
    Abstract

    Core–shell structured ZIF-8@ZIF-67 crystals are well-designed and prepared through a seed-mediated growth method. After thermal treatment of ZIF-8@ZIF-67 crystals, we obtain selectively functionalized nanoporous hybrid carbon materials consisting of nitrogen-doped carbon (NC) as the cores and highly graphitic carbon (GC) as the shells. This is the first example of the integration of NC and GC in one particle at the nanometer level. Electrochemical data strongly demonstrate that this nanoporous hybrid carbon material integrates the advantageous properties of the individual NC and GC, exhibiting a distinguished specific capacitance (270 F·g–1) calculated from the galvanostatic charge–discharge curves at a current density of 2 A·g–1. Our study not only bridges diverse carbon-based materials with infinite metal–organic frameworks but also opens a new avenue for artificially designed nanoarchitectures with target functionalities.

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