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    The application of synchrotron methods in characterizing iron and cobalt Fischer-Tropsch synthesis catalysts

    Access Status
    Fulltext not available
    Authors
    Jacobs, G.
    Ma, W.
    Gao, P.
    Todic, B.
    Bhatelia, Tejas
    Bukur, D.
    Davis, B.
    Date
    2013
    Type
    Journal Article
    
    Metadata
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    Citation
    Jacobs, G. and Ma, W. and Gao, P. and Todic, B. and Bhatelia, T. and Bukur, D. and Davis, B. 2013. The application of synchrotron methods in characterizing iron and cobalt Fischer-Tropsch synthesis catalysts. Catalysis Today. 214: pp. 100-139.
    Source Title
    Catalysis Today
    DOI
    10.1016/j.cattod.2013.05.011
    ISSN
    0920-5861
    URI
    http://hdl.handle.net/20.500.11937/63340
    Collection
    • Curtin Research Publications
    Abstract

    This article reviews the use of synchrotron radiation techniques to confront issues associated with cobalt and iron catalysts. The main areas that are examined include: (1) the application of TPR-XANES and TPR-EXAFS to gain insight into the hydrogen reduction of cobalt catalysts and the carburization of iron catalysts; (2) the impact of promoters on these reduction/carburization rates; (3) the local atomic structure of promoters and its influence on catalyst selectivity; (4) exploring the deactivation of cobalt catalysts; (5) the influence of crystallite size in stabilizing cobalts catalyst against water effects; and (6) temperature effects in alkali promoted iron catalysts in retaining the iron carbide phase against reoxidation by water. © 2012 Elsevier B.V. All rights reserved.

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