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dc.contributor.authorTian, W.
dc.contributor.authorZhang, H.
dc.contributor.authorSun, Hongqi
dc.contributor.authorTade, Moses
dc.contributor.authorWang, Shaobin
dc.date.accessioned2018-02-06T06:17:01Z
dc.date.available2018-02-06T06:17:01Z
dc.date.created2018-02-06T05:49:54Z
dc.date.issued2017
dc.identifier.citationTian, W. and Zhang, H. and Sun, H. and Tade, M. and Wang, S. 2017. Template-free synthesis of N-doped carbon with pillared-layered pores as bifunctional materials for supercapacitor and environmental applications. Carbon. 118: pp. 98-105.
dc.identifier.urihttp://hdl.handle.net/20.500.11937/63374
dc.identifier.doi10.1016/j.carbon.2017.03.027
dc.description.abstract

© 2017 Elsevier Ltd Cross-linked, N-doped, pillared-layered porous carbons (NCs) were prepared via a one-pot, template-free pyrolysis process at 600 (NC600), 700 (NC700) and 800 °C (NC800), which have bifunctional applications in supercapacitors and environmental remediation. NC700 displays a high surface area (2118 m 2  g −1 ) and a specific capacitance of 305 F g −1  at 0.2 A g −1 in a two-electrode setup. The maximum energy density of NC700 was 20.4 W h/kg at a power density of 139 W kg −1 and 89.1% capacitance was retained after 10000 cycles of charge-discharge at 5 A g −1 . For water remediation, NC800 displayed high adsorption capacities towards flame retardant tetrabromobisphenol A (TBBPA, 372  mg g −1 ) and antibiotic sulfachloropyridazine (SCP, 288 mg g −1 ) solutions, while NC700 showed the most efficient SCP oxidation removal. These results suggest low-cost and green carbon materials as electrodes in flexible energy storage devices, metal-free adsorbents as well as catalysts for high efficient removal of emerging contaminants in aqueous solution.

dc.publisherPergamon
dc.relation.sponsoredbyhttp://purl.org/au-research/grants/arc/DP130101319
dc.relation.sponsoredbyhttp://purl.org/au-research/grants/arc/DP150103026
dc.titleTemplate-free synthesis of N-doped carbon with pillared-layered pores as bifunctional materials for supercapacitor and environmental applications
dc.typeJournal Article
dcterms.source.volume118
dcterms.source.startPage98
dcterms.source.endPage105
dcterms.source.issn0008-6223
dcterms.source.titleCarbon
curtin.departmentDepartment of Chemical Engineering
curtin.accessStatusFulltext not available


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