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    Recent progress in metal–organic frameworks for lithium–sulfur batteries

    71031.pdf (1.865Mb)
    Access Status
    Open access
    Authors
    Zhong, Y.
    Xu, X.
    Liu, Y.
    Wang, W.
    Shao, Zongping
    Date
    2018
    Type
    Journal Article
    
    Metadata
    Show full item record
    Citation
    Zhong, Y. and Xu, X. and Liu, Y. and Wang, W. and Shao, Z. 2018. Recent progress in metal–organic frameworks for lithium–sulfur batteries. Polyhedron. 155: pp. 464-484.
    Source Title
    Polyhedron
    DOI
    10.1016/j.poly.2018.08.067
    ISSN
    0277-5387
    School
    WASM: Minerals, Energy and Chemical Engineering (WASM-MECE)
    Funding and Sponsorship
    http://purl.org/au-research/grants/arc/DP150104365
    http://purl.org/au-research/grants/arc/DP160104835
    URI
    http://hdl.handle.net/20.500.11937/70788
    Collection
    • Curtin Research Publications
    Abstract

    © 2018 Elsevier Ltd The development of novel electrochemical energy storage systems has induced a great evolution of sustainable production and life. Lithium–sulfur (Li–S) batteries show a significant potential of becoming the next-generation energy storage systems, even though several vital problems, especially the dissolution and loss of active polysulfides, still hinder their practical application. Metal–organic frameworks (MOFs), a novel class of porous crystalline materials, and their derived materials, exhibit great potential for anchoring soluble polysulfides due to the unique physical and surface chemical property. In this review, we dedicate to review strategies for designing MOF-based and MOF-derived materials as hosts and functional polysulfide barriers for Li–S batteries. By revisiting three most important parameters for the design of hosts, namely conductivity, porosity and chemisorption to polysulfides, we hope to gain a greater understanding of how these MOF-related materials promote the electrochemical performance and the cycle stability of Li–S batteries. We also summarize the recent advances of two types of polysulfide barriers working based on an adsorbing-reutilization approach and a blocking approach. Finally, we point out the main challenges and some perspectives for the future development of this promising area.

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