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dc.contributor.authorLiu, Jian
dc.contributor.authorHuang, J.
dc.contributor.authorZhou, H.
dc.contributor.authorAntonietti, M.
dc.date.accessioned2018-12-13T09:13:39Z
dc.date.available2018-12-13T09:13:39Z
dc.date.created2018-12-12T02:46:47Z
dc.date.issued2014
dc.identifier.citationLiu, J. and Huang, J. and Zhou, H. and Antonietti, M. 2014. Uniform graphitic carbon nitride nanorod for efficient photocatalytic hydrogen evolution and sustained photoenzymatic catalysis. ACS Applied Materials and Interfaces. 6 (11): pp. 8434-8440.
dc.identifier.urihttp://hdl.handle.net/20.500.11937/72529
dc.identifier.doi10.1021/am501319v
dc.description.abstract

Uniform graphitic carbon nitride nanorods (CNR) were facilely obtained by a morphology-preserving strategy by templating a chiral mesostructured silica nanorod. The hexagonal mesostructured pore structures of one-dimensional silica nanorods can provide nanoconfinement space for carbon nitride condensation to perfect layered structures. CNR demonstrated excellent photocatalytic capability in generating hydrogen from water even with a small specific surface area, compared with its mesoporous counterpart. For further application demonstration, the CNR was used for photocatalytic regeneration of NAD+ to NADH, the biological form of hydrogen. The in situ NADH regeneration system was further coupled with l-glutamate dehydrogenase for sustainable generation of l-glutamate from a-ketoglutarate. The high yield and high efficiency obtained here point a high-throughput and sustainable way for practical enzymatic applications. © 2014 American Chemical Society.

dc.publisherAmerican Chemical Society
dc.titleUniform graphitic carbon nitride nanorod for efficient photocatalytic hydrogen evolution and sustained photoenzymatic catalysis
dc.typeJournal Article
dcterms.source.volume6
dcterms.source.number11
dcterms.source.startPage8434
dcterms.source.endPage8440
dcterms.source.issn1944-8244
dcterms.source.titleACS Applied Materials and Interfaces
curtin.departmentWASM: Minerals, Energy and Chemical Engineering (WASM-MECE)
curtin.accessStatusFulltext not available


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