Hybrid C<inf>3</inf>N<inf>4</inf>/Fluorine-Doped Tin Oxide Electrode Transfers Hydride for 1,4-NADH Cofactor Regeneration
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© 2015 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim. Herein, we report the use of graphitic carbon nitride (C<inf>3</inf>N<inf>4</inf>)-modified fluorine-doped tin oxide electrodes for the electroregeneration of reduced nicotinamide adenine dinucleotide phosphate (NADH). We synthesized and functionalized these hybrid electrodes by using anodic aluminum-oxide-templated C<inf>3</inf>N<inf>4</inf> growth. Electrochemical activation of the semiconducting C<inf>3</inf>N<inf>4</inf> islands with a rhodium complex permits selective regeneration of biologically active 1,4-NADH cofactor. A ride for the hydride: Graphitic carbon nitride (C<inf>3</inf>N<inf>4</inf>)-modified fluorine-doped tin oxide (FTO) electrodes are used for the electroregeneration of reduced nicotinamide adenine dinucleotide phosphate (NADH). These hybrid electrodes are synthesized by using anodic aluminum-oxide-templated C<inf>3</inf>N<inf>4</inf> growth. Electrochemical activation of the semiconducting C<inf>3</inf>N<inf>4</inf> islands with a rhodium complex permits selective regeneration of biologically active 1,4-NADH cofactor.
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