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    Polymorphism and its effects on the magnetic behaviour of the [Fe(sal2-trien)][Ni(dmit)2] spin-crossover complex

    Access Status
    Fulltext not available
    Authors
    Faulmann, C.
    Szilagyi, Petra
    Jacob, K.
    Chahine, J.
    Valade, L.
    Date
    2009
    Type
    Journal Article
    
    Metadata
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    Citation
    Faulmann, C. and Szilagyi, P. and Jacob, K. and Chahine, J. and Valade, L. 2009. Polymorphism and its effects on the magnetic behaviour of the [Fe(sal2-trien)][Ni(dmit)2] spin-crossover complex. New Journal of Chemistry. 33: pp. 1268-1276.
    Source Title
    New Journal of Chemistry
    Additional URLs
    http://pubs.rsc.org/en/Content/ArticleLanding/2009/NJ/b901779h#!divAbstract
    ISSN
    1144-0546
    URI
    http://hdl.handle.net/20.500.11937/9447
    Collection
    • Curtin Research Publications
    Abstract

    The syntheses, structural characterisation, and magnetic and spectroscopic properties of three new polymorphs of the spin-crossover complex [Fe(sal2-trien)][Ni(dmit)2] are reported. The results are discussed as a function of their intra- and intermolecular arrangement. Correlation of their crystal structures and magnetic properties suggest that some torsion angles play a significant role in the magnetic properties of this class of compounds. Intermolecular contacts are also of importance, and the nature of the short contacts between molecular species seems to be more crucial than their number in the allowance of spin-crossover.

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