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    Volume-Based Thermoelasticity: Consequences of the (Near) Proportionality of Isothermal Compressibility to Formula-Unit Volume

    Access Status
    Fulltext not available
    Authors
    Jenkins, H.
    Glasser, Leslie
    Lee, J.
    Date
    2010
    Type
    Journal Article
    
    Metadata
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    Citation
    Jenkins, H. Donald and Glasser, Leslie and Lee, Joe. 2010. Volume-Based Thermoelasticity: Consequences of the (Near) Proportionality of Isothermal Compressibility to Formula-Unit Volume. Inorganic Chemistry. 49 (21): pp. 9978-9984.
    Source Title
    Inorganic Chemistry
    DOI
    10.1021/ic101398g
    ISSN
    00201669
    Faculty
    Nanochemistry Research Institute (NRI)
    Faculty of Science and Engineering
    School
    Nanochemistry Research Institute (Research Institute)
    URI
    http://hdl.handle.net/20.500.11937/14278
    Collection
    • Curtin Research Publications
    Abstract

    Groups of structurally related materials, including the alkali halides, exhibit a proportionality of isothermal compressibility to formula-unit volume. The relationship has recently been explored by Glasser and by Recio et al. In this paper, we present the consequences of such proportionality on the relationships of Born-Lande and Born-Mayer parameters to the formula-unit volume. These relationships have then been tested separately on (i) alkali (excluding cesium) halides and (ii) cesium halides.We conclude that the equations fit the NaCl-type materials satisfactorily, but less well for the CsCl-type materials, and that the Born-Mayer equation is more applicable. These results confirm the conclusion that volume is intimately linked to thermodynamic quantities, as already demonstrated by our development of volume-based thermodynamics (VBT).

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