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    Divergent synthesis of ruthenium alkynyl dendrimers and a two-photon absorption cross-section dendritic effect

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    Authors
    Green, K.
    Simpson, Peter
    Corkery, T.
    Cifuentes, M.
    Samoc, M.
    Humphrey, M.
    Date
    2012
    Type
    Journal Article
    
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    Citation
    Green, K. and Simpson, P. and Corkery, T. and Cifuentes, M. and Samoc, M. and Humphrey, M. 2012. Divergent synthesis of ruthenium alkynyl dendrimers and a two-photon absorption cross-section dendritic effect. Macromolecular Rapid Communications. 33 (6-7): pp. 573-578.
    Source Title
    Macromolecular Rapid Communications
    DOI
    10.1002/marc.201100770
    ISSN
    1022-1336
    School
    Nanochemistry Research Institute
    URI
    http://hdl.handle.net/20.500.11937/22475
    Collection
    • Curtin Research Publications
    Abstract

    Ruthenium alkynyl dendrimers up to second generation in size have been prepared by a divergent route and exploiting Sonogashira coupling. The cubic NLO properties have been examined by wide spectral range fs Z-scan studies, revealing an NLO dendritic effect. The significant increase in NLO properties seen on generation increase is maintained when the coefficients are scaled by the number of metal atoms, the dendrimer molecular weights, or the number of "effective" (delocalizable p) electrons in the dendritic structures. © 2012 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

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